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Non-Equilibrium Charge Motion in Organic Solar Cells
Organic photovoltaic (OPV) devices based on semiconducting polymers and small molecules allow for a low cost alternative to inorganic solar cells. Recent developments show power conversion efficiencies as high as 10-12%, highlighting the potential of this technology. Nevertheless, further improvements are necessary to achieve commercialization. To a large extent the performance of these devices is dictated by their ability to extract the photo-generated charge, which is related to the charge carrier mobility. Various time-resolved and steady-state techniques are available to probe the charge carrier mobility in OPVs but often lead to different mobility values for one and the same system. Des...
Effects of Energetic Disorder on the Optoelectronic Properties of Organic Solar Cells
Organic photovoltaics (OPVs) is a promising low-cost and environmental-friendly technology currently achieving 12-14% power conversion efficiency. Despite the extensive focus of the research community over the last years, critical mechanisms defining the performance of OPVs are still topics of debate. While energetic disorder is known to be characteristic of organic semiconductors in general, its potential role in OPV has received surprisingly little attention. In this thesis we investigate some aspects of the relation between energetic disorder and several optoelectronic properties of OPV. Charge carrier mobility is a key parameter in characterizing the performance of organic semiconductors...
Organic Solar Cells
This book covers in a textbook-like fashion the basics or organic solar cells, addressing the limits of photovoltaic energy conversion and giving a well-illustrated introduction to molecular electronics with focus on the working principle and characterization of organic solar cells. Further chapters based on the author’s dissertation focus on the electrical processes in organic solar cells by presenting a detailed drift-diffusion approach to describe exciton separation and charge-carrier transport and extraction. The results, although elaborated on small-molecule solar cells and with focus on the zinc phthalocyanine: C60 material system, are of general nature. They propose and demonstrate ...
Multifunctional Supramolecular Organic Ferroelectrics
Ferroelectric materials are known and valued for their multifunctionality arising from the possibility to perturb the remnant ferroelectric polarization by electric field, temperature and/or mechanical stimuli. While inorganic ferroelectrics dominate the current market, their organic counterparts may provide highly desired properties like eco-friendliness, easy processability and flexibility, concomitantly opening unique opportunities to combine multiple functionalities into a single compound that facilitates unprecedented device concepts and designs. Supramolecular organic ferroelectrics of columnar discotic type, that are the topic of this thesis, offer additional advantages related to the...
Polymer/polymer blends in organic photovoltaic and photodiode devices
Organic photovoltaics devices (OPV) have attracted attentions of scientist for their potential as inexpensive, lightweight, flexible and suitable for roll-to-roll production. In recent years, considerable attention has been focused on new acceptor materials, either polymeric or small molecules, to replace the once dominating fullerene derivatives. The emergence of numerous new non-fullerene materials has driven power conversion efficiency (PCE) up to 17%, attracting more and more interests of commercialization. Polymer acceptors with more morphology stability, more absorption and more desired energy levels has been intensively studied and show great potential for large area and low-cost prod...
Polymers in Electronics
Polymers in Electronics: Optoelectronic Properties, Design, Fabrication, and Applications brings together the fundamentals and latest advances in polymeric materials for electronic device applications, supporting researchers, scientists and advanced students, and approaching the topic from a range of disciplines. The book begins by introducing polymeric materials, their dielectric, optical, and thermal properties, and the essential principles and techniques for polymers as applied to electronics. This is followed by detailed coverage of the key steps in the preparation of polymeric materials for opto-electronic devices, including fabrication methods, materials design, rheology, encapsulation...
Doping and Density of States Engineering for Organic Thermoelectrics
Thermoelectric materials can turn temperature differences directly into electricity. To use this to harvest e.g. waste heat with an efficiency that approaches the Carnot efficiency requires a figure of merit ZT larger than 1. Compared with their inorganic counterparts, organic thermoelectrics (OTE) have numerous advantages, such as low cost, large-area compatibility, flexibility, material abundance and an inherently low thermal conductivity. Therefore, organic thermoelectrics are considered by many to be a promising candidate material system to be used in lower cost and higher efficiency thermoelectric energy conversion, despite record ZT values for OTE currently lying around 0.25. A complet...
Local Activity Principle: The Cause Of Complexity And Symmetry Breaking
The principle of local activity explains the emergence of complex patterns in a homogeneous medium. At first defined in the theory of nonlinear electronic circuits in a mathematically rigorous way, it can be generalized and proven at least for the class of nonlinear reaction-diffusion systems in physics, chemistry, biology, and brain research. Recently, it was realized by memristors for nanoelectronic device applications. In general, the emergence of complex patterns and structures is explained by symmetry breaking in homogeneous media, which is caused by local activity. This book argues that the principle of local activity is really fundamental in science, and can even be identified in quantum cosmology as symmetry breaking of local gauge symmetries generating the complexity of matter and forces in our universe. Applications are considered in economic, financial, and social systems with the emergence of equilibrium states, symmetry breaking at critical points of phase transitions and risky acting at the edge of chaos./a
Mathematical Foundations of Neuroscience
This book applies methods from nonlinear dynamics to problems in neuroscience. It uses modern mathematical approaches to understand patterns of neuronal activity seen in experiments and models of neuronal behavior. The intended audience is researchers interested in applying mathematics to important problems in neuroscience, and neuroscientists who would like to understand how to create models, as well as the mathematical and computational methods for analyzing them. The authors take a very broad approach and use many different methods to solve and understand complex models of neurons and circuits. They explain and combine numerical, analytical, dynamical systems and perturbation methods to p...
